Cobalt(II) bromide

Cobalt(II) bromide
Structure of cobalt(II) bromide tetrahydrate
Crystal structure of cobalt(II) bromide
Anhydrous cobalt(II) bromide in a vial
Identifiers
3D model (JSmol)
ChemSpider
ECHA InfoCard 100.029.242
EC Number
  • 232-166-7
RTECS number
  • GF9595000
UNII
UN number 3077
  • InChI=1S/2BrH.Co/h2*1H;/q;;+2/p-2 Y
    Key: BZRRQSJJPUGBAA-UHFFFAOYSA-L Y
  • InChI=1/2BrH.Co/h2*1H;/q;;+2/p-2
    Key: BZRRQSJJPUGBAA-NUQVWONBAJ
  • [Co](Br)Br
Properties
CoBr2, CoBr2.6H2O, CoBr2.2H2O
Molar mass 218.7412 g/mol (anhydrous)
326.74 g/mol (hexahydrate)
Appearance Bright green crystals (anhydrous)
Red-purple crystals (hexahydrate)
Density 4.909 g/cm3 (anhydrous)
2.46 g/cm3 (hexahydrate)
Melting point 678 °C (1,252 °F; 951 K) (anhydrous)[1][2]
47 °C (hexahydrate)
anhydrous:
66.7 g/100 mL (59 °C)
68.1 g/100 mL (97 °C)
hexahydrate:
113.2 g/100 mL (20 °C)
Solubility 77.1 g/100 mL (ethanol, 20 °C)
58.6 g/100 mL (methanol, 30 °C)
soluble in methyl acetate, ether, alcohol, acetone
+13000·10−6 cm3/mol
Structure
Rhombohedral, hP3, SpaceGroup = P-3m1, No. 164
octahedral
Hazards
GHS labelling:
Danger
H302, H312, H315, H317, H319, H332, H334, H335, H350
P201, P202, P261, P264, P270, P271, P272, P280, P281, P285, P301+P312, P302+P352, P304+P312, P304+P340, P304+P341, P305+P351+P338, P308+P313, P312, P321, P322, P330, P332+P313, P333+P313, P337+P313, P342+P311, P362, P363, P403+P233, P405, P501
NFPA 704 (fire diamond)
2
0
1
Flash point Non-flammable
Lethal dose or concentration (LD, LC):
406 mg/kg (oral, rat)
Safety data sheet (SDS) Fisher Scientific
Related compounds
Other anions
cobalt(II) fluoride
cobalt(II) chloride
cobalt(II) iodide
Other cations
iron(II) bromide
nickel(II) bromide
Except where otherwise noted, data are given for materials in their standard state (at 25 °C [77 °F], 100 kPa).
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Infobox references

Cobalt(II) bromide refers to inorganic compounds with the formula CoBr2·(H2O)n. The anhydrous form (n = 0) is a green solid and the hexahydrate (n = 6) is a red solid.[3] These compounds find some use as catalysts.[4]

Structure

The anhydrous compound has a cadmium iodide structure. The tetrahydrate is molecular, with the formula trans-[CoBr2(H2O)4].[5]

Preparation and reactions

Cobalt(II) bromide form by treating an aqueous suspension of cobalt(II) carbonate with hydrobromic acid according to the following idealized equation:[3]

CoCO3 + 2 HBr + 5 H2O → CoBr2(H2O)6 + CO2

Anhydrous cobalt(II) bromide is hygroscopic. Air exposure eventually forms the hexahydrate in air,[6] which appears as red-purple crystals. The hexahydrate loses four water of crystallization molecules at 100 °C forming the dihydrate:

CoBr2·6H2O → CoBr2·2H2O + 4 H2O

The anhydrous compound forms by heating any of the hydrates to >150 °C in a vacuum:

CoBr2(H2O)6 → CoBr2 + 6 H2O

The resulting solid can be purified by vacuum sublimation at > 500 °C.[3]

Further heating to 130 °C produces the anhydrous form:

CoBr2·2H2O → CoBr2 + 2 H2O

At higher temperatures, cobalt(II) bromide reacts with oxygen, forming cobalt(II,III) oxide and bromine vapor.

The coordination compound bromopentaamminecobalt(III) bromide is prepared by oxidation of an aqueous solution of cobalt(II) bromide and ammonia.[7]

2 CoBr2 + 8 NH3 + 2 NH4Br + H2O2 → 2 [Co(NH3)5Br]Br2 + 2 H2O

Triphenylphosphine complexes of cobalt(II) bromide have been used as a catalysts in organic synthesis.[8]

Safety

Exposure to large amounts of cobalt(II) can cause cobalt poisoning.[9] Bromide is also mildly toxic.

References

  1. ^ Cobalt Bromide Supplier & Tech Info American Elements
  2. ^ WebElements Periodic Table of the Elements
  3. ^ a b c O. Glemser (1963). "Cobalt(II) bromide". In G. Brauer (ed.). Handbook of Preparative Inorganic Chemistry, 2nd Ed. Vol. 2. NY, NY: Academic Press. p. 1517.
  4. ^ Le Gall, Erwan; Martens, Thierry (2012). "Multicomponent Synthesis of Tertiary Diarylmethylamines: 1-((4-Fluorophenyl)(4-methoxyphenyl)methyl)piperidine". Organic Syntheses. 89: 283. doi:10.15227/orgsyn.089.0283.
  5. ^ Waizumi, Kenji; Masuda, Hideki; Ohtaki, Hitoshi (1992). "X-ray Structural Studies of FeBr2·4H2O, CoBr2·4H2O, NiCl2·4H2O and CuBr2·4H2O. Cis/Trans Selectivity in Transition Metal(II) Dihalide Tetrahydrate". Inorganica Chimica Acta. 192 (2): 173–181. doi:10.1016/S0020-1693(00)80756-2.
  6. ^ Perry, Dale L. (2011). Handbook of Inorganic Compounds (2nd ed.). Boca Raton: Taylor & Francis. p. 130. ISBN 978-1-4398-1461-1. OCLC 587104373.
  7. ^ Diehl, Harvey; Clark, Helen; Willard, H. H.; Bailar, John C. (1939). "Bromopentamminocobalti Bromide". Inorganic Syntheses. Vol. 1. p. 186. doi:10.1002/9780470132326.ch66. ISBN 978-0-470-13232-6. {{cite book}}: ISBN / Date incompatibility (help)
  8. ^ Gund, Tamara M.; Thielecke, Wilfried; R. Schleyer, Paul v. (1973). "Diamantane: Pentacyclo[7.3.1.14,12.02,7.06,11]Tetradecane". Organic Syntheses. 53: 30. doi:10.15227/orgsyn.053.0030.
  9. ^ "Cobalt Bromide (OUS)" (PDF). Archived from the original (PDF) on 2007-06-25. Retrieved 2008-04-10.